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DOI | 10.1126/science.aam7092 |
Perovskites in catalysis and electrocatalysis | |
Hwang, Jonathan1; Rao, Reshma R.2; Giordano, Livia2,3; Katayama, Yu4,5; Yu, Yang1; Shao-Horn, Yang1,2,4 | |
2017-11-10 | |
发表期刊 | SCIENCE |
ISSN | 0036-8075 |
EISSN | 1095-9203 |
出版年 | 2017 |
卷号 | 358期号:6364页码:751-756 |
文章类型 | Review |
语种 | 英语 |
国家 | USA; Italy; Japan |
英文摘要 | Catalysts for chemical and electrochemical reactions underpin many aspects of modern technology and industry, from energy storage and conversion to toxic emissions abatement to chemical and materials synthesis. This role necessitates the design of highly active, stable, yet earth-abundant heterogeneous catalysts. In this Review, we present the perovskite oxide family as a basis for developing such catalysts for (electro)chemical conversions spanning carbon, nitrogen, and oxygen chemistries. A framework for rationalizing activity trends and guiding perovskite oxide catalyst design is described, followed by illustrations of how a robust understanding of perovskite electronic structure provides fundamental insights into activity, stability, and mechanism in oxygen electrocatalysis. We conclude by outlining how these insights open experimental and computational opportunities to expand the compositional and chemical reaction space for next-generation perovskite catalysts. |
领域 | 地球科学 ; 气候变化 ; 资源环境 |
收录类别 | SCI-E |
WOS记录号 | WOS:000414847100037 |
WOS关键词 | TRANSITION-METAL OXIDES ; RAY PHOTOELECTRON-SPECTROSCOPY ; CARBON-MONOXIDE OXIDATION ; OXYGEN-EVOLUTION ; CO OXIDATION ; IN-SITU ; WATER OXIDATION ; FUEL-CELLS ; ABSORPTION SPECTROSCOPY ; NO OXIDATION |
WOS类目 | Multidisciplinary Sciences |
WOS研究方向 | Science & Technology - Other Topics |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/197298 |
专题 | 地球科学 资源环境科学 气候变化 |
作者单位 | 1.MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA; 2.MIT, Dept Mech Engn, Cambridge, MA 02139 USA; 3.Univ Milano Bicocca, Dept Mat Sci, Via Cozzi 55, I-20136 Milan, Italy; 4.MIT, Res Lab Elect, 77 Massachusetts Ave, Cambridge, MA 02139 USA; 5.Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Kyoto 6158510, Japan |
推荐引用方式 GB/T 7714 | Hwang, Jonathan,Rao, Reshma R.,Giordano, Livia,et al. Perovskites in catalysis and electrocatalysis[J]. SCIENCE,2017,358(6364):751-756. |
APA | Hwang, Jonathan,Rao, Reshma R.,Giordano, Livia,Katayama, Yu,Yu, Yang,&Shao-Horn, Yang.(2017).Perovskites in catalysis and electrocatalysis.SCIENCE,358(6364),751-756. |
MLA | Hwang, Jonathan,et al."Perovskites in catalysis and electrocatalysis".SCIENCE 358.6364(2017):751-756. |
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