GSTDTAP  > 地球科学
DOI10.5194/acp-18-691-2018
MLS measurements of stratospheric hydrogen cyanide during the 2015-2016 El Nino event
Pumphrey, Hugh C.1; Glatthor, Norbert2; Bernath, Peter F.3,4; Boone, Christopher D.4; Hannigan, James W.5; Ortega, Ivan5; Livesey, Nathaniel J.6; Read, William G.6
2018-01-19
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:2页码:691-703
文章类型Article
语种英语
国家Scotland; Germany; USA; Canada
英文摘要

It is known from ground-based measurements made during the 1982-1983 and 1997-1998 El Nino events that atmospheric hydrogen cyanide (HCN) tends to be higher during such years than at other times. The Microwave Limb Sounder (MLS) on the Aura satellite has been measuring HCN mixing ratios since launch in 2004; the measurements are ongoing at the time of writing. The winter of 20152016 saw the largest El Nino event since 1997-1998. We present MLS measurements of HCN in the lower stratosphere for the Aura mission to date, comparing the 20152016 El Nino period to the rest of the mission. HCN in 20152016 is higher than at any other time during the mission, but ground-based measurements suggest that it may have been even more elevated in 1997-1998. As the MLS HCN data are essentially unvalidated, we show them alongside data from the MIPAS and ACE-FTS instruments; the three instruments agree reasonably well in the tropical lower stratosphere. Global HCN emissions calculated from the Global Fire Emissions Database (GFED v4.1) database are much greater during large El Nino events and are greater in 19971998 than in 2015-2016, thereby showing good qualitative agreement with the measurements. Correlation between El Nino-Southern Oscillation (ENSO) indices, measured HCN, and GFED HCN emissions is less clear if the 2015-2016 event is excluded. In particular, the 2009-2010 winter had fairly strong El Nino conditions and fairly large GFED HCN emissions, but very little effect is observed in the MLS HCN.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000423021000001
WOS关键词FREE TROPOSPHERIC CO ; ATMOSPHERIC CHEMISTRY ; SOUTHERN-OSCILLATION ; EQUATORIAL PACIFIC ; EOS MLS ; HCN ; TRANSPORT ; POLLUTION ; FIRES ; EMISSIONS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/19531
专题地球科学
作者单位1.Univ Edinburgh, Sch GeoSci, Edinburgh, Midlothian, Scotland;
2.Karlsruher Inst Technol, Inst Meteorol & Klimaforsch, Karlsruhe, Germany;
3.Old Dominion Univ, Dept Chem & Biochem, Norfolk, VA 23508 USA;
4.Univ Waterloo, Dept Chem, Waterloo, ON N2L 3G1, Canada;
5.Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA;
6.CALTECH, Jet Prop Lab, NASA, Pasadena, CA USA
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Pumphrey, Hugh C.,Glatthor, Norbert,Bernath, Peter F.,et al. MLS measurements of stratospheric hydrogen cyanide during the 2015-2016 El Nino event[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(2):691-703.
APA Pumphrey, Hugh C..,Glatthor, Norbert.,Bernath, Peter F..,Boone, Christopher D..,Hannigan, James W..,...&Read, William G..(2018).MLS measurements of stratospheric hydrogen cyanide during the 2015-2016 El Nino event.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(2),691-703.
MLA Pumphrey, Hugh C.,et al."MLS measurements of stratospheric hydrogen cyanide during the 2015-2016 El Nino event".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.2(2018):691-703.
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