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DOI | 10.1126/science.aad4998 |
Combining theory and experiment in electrocatalysis: Insights into materials design | |
Seh, Zhi Wei1,2,3; Kibsgaard, Jakob1,2,4; Dickens, Colin F.1,2; Chorkendorff, I. B.4; Norskov, Jens K.1,2; Jaramillo, Thomas F.1,2 | |
2017-01-13 | |
发表期刊 | SCIENCE
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ISSN | 0036-8075 |
EISSN | 1095-9203 |
出版年 | 2017 |
卷号 | 355期号:6321 |
文章类型 | Review |
语种 | 英语 |
国家 | USA; Singapore; Denmark |
英文摘要 | Electrocatalysis plays a central role in clean energy conversion, enabling a number of sustainable processes for future technologies. This review discusses design strategies for state-of-the-art heterogeneous electrocatalysts and associated materials for several different electrochemical transformations involving water, hydrogen, and oxygen, using theory as a means to rationalize catalyst performance. By examining the common principles that govern catalysis for different electrochemical reactions, we describe a systematic framework that clarifies trends in catalyzing these reactions, serving as a guide to new catalyst development while highlighting key gaps that need to be addressed. We conclude by extending this framework to emerging clean energy reactions such as hydrogen peroxide production, carbon dioxide reduction, and nitrogen reduction, where the development of improved catalysts could allow for the sustainable production of a broad range of fuels and chemicals. |
领域 | 地球科学 ; 气候变化 ; 资源环境 |
收录类别 | SCI-E |
WOS记录号 | WOS:000391743700032 |
WOS关键词 | HYDROGEN-EVOLUTION REACTION ; OXYGEN REDUCTION REACTION ; PEROVSKITE OXIDE CATALYSTS ; DENSITY-FUNCTIONAL THEORY ; NITROGEN-DOPED CARBON ; ACTIVE EDGE SITES ; ELECTROCHEMICAL REDUCTION ; WATER OXIDATION ; METAL-SURFACES ; PHOSPHIDE NANOPARTICLES |
WOS类目 | Multidisciplinary Sciences |
WOS研究方向 | Science & Technology - Other Topics |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/195227 |
专题 | 地球科学 资源环境科学 气候变化 |
作者单位 | 1.Stanford Univ, Dept Chem Engn, SUNCAT Ctr Interface Sci & Catalysis, Stanford, CA 94305 USA; 2.SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA; 3.ASTAR, Inst Mat Res & Engn, Innovis 138634, Singapore; 4.Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark |
推荐引用方式 GB/T 7714 | Seh, Zhi Wei,Kibsgaard, Jakob,Dickens, Colin F.,et al. Combining theory and experiment in electrocatalysis: Insights into materials design[J]. SCIENCE,2017,355(6321). |
APA | Seh, Zhi Wei,Kibsgaard, Jakob,Dickens, Colin F.,Chorkendorff, I. B.,Norskov, Jens K.,&Jaramillo, Thomas F..(2017).Combining theory and experiment in electrocatalysis: Insights into materials design.SCIENCE,355(6321). |
MLA | Seh, Zhi Wei,et al."Combining theory and experiment in electrocatalysis: Insights into materials design".SCIENCE 355.6321(2017). |
条目包含的文件 | 条目无相关文件。 |
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