GSTDTAP  > 地球科学
DOI10.5194/acp-19-11279-2019
Analysis of total column CO2 and CH4 measurements in Berlin with WRF-GHG
Zhao, Xinxu1; Marshall, Julia2; Hachinger, Stephan3; Gerbig, Christoph2; Frey, Matthias4; Hase, Frank4; Chen, Jia1
2019-09-06
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:17页码:11279-11302
文章类型Article
语种英语
国家Germany
英文摘要

Though they cover less than 3% of the global land area, urban areas are responsible for over 70% of the global greenhouse gas (GHG) emissions and contain 55% of the global population. A quantitative tracking of GHG emissions in urban areas is therefore of great importance, with the aim of accurately assessing the amount of emissions and identifying the emission sources. The Weather Research and Forecasting model (WRF) coupled with GHG modules (WRFGHG) developed for mesoscale atmospheric GHG transport can predict column-averaged abundances of CO2 and CH4 (XCO2 and XCH4). In this study, we use WRF-GHG to model the Berlin area at a high spatial resolution of 1 km. The simulated wind and concentration fields were compared with the measurements from a campaign performed around Berlin in 2014 (Hase et al., 2015). The measured and simulated wind fields mostly demonstrate good agreement. The simulated XCO2 shows quite similar trends with the measurement but with approximately 1 ppm bias, while a bias in the simulated XCH4 of around 2.7% is found. The bias could potentially be the result of relatively high background concentrations, the errors at the tropopause height, etc. We find that an analysis using differential column methodology (DCM) works well for the XCH4 comparison, as corresponding background biases are then canceled out. From the tracer analysis, we find that the enhancement of XCH4 is highly dependent on human activities. The XCO2 enhancement in the vicinity of Berlin is dominated by anthropogenic behavior rather than biogenic activities. We conclude that DCM is an effective method for comparing models to observations independently of biases caused, e.g., by initial conditions. It allows us to use our high-resolution WRF-GHG model to detect and understand major sources of GHG emissions in urban areas.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000484560600002
WOS关键词PORTABLE FTIR SPECTROMETERS ; METHANE EMISSIONS ; ERROR CHARACTERIZATION ; GREENHOUSE GASES ; TRANSPORT MODELS ; ATMOSPHERIC CO2 ; EUROPEAN CH4 ; QUANTIFICATION ; SIMULATIONS ; CONSISTENCY
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/186946
专题地球科学
作者单位1.Tech Unversitat Munchen, Dept Elect & Comp Engn, Arcisstr 21, D-80333 Munich, Germany;
2.Max Planck Inst Biogeochem, Dept Biogeochem Syst, Hans Knoll Str 10, D-07745 Jena, Germany;
3.Bavarian Acad Sci & Humanities, Leibniz Rechenzenturm LRZ, Leibniz Supercomp Ctr, Bolzmannstr 1, D-85748 Garching, Germany;
4.KIT, Inst Meteorol & Climate Res IMK ASF, Hermann von Helmholtz Pl 1, D-76021 Karlsruhe, Germany
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GB/T 7714
Zhao, Xinxu,Marshall, Julia,Hachinger, Stephan,et al. Analysis of total column CO2 and CH4 measurements in Berlin with WRF-GHG[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(17):11279-11302.
APA Zhao, Xinxu.,Marshall, Julia.,Hachinger, Stephan.,Gerbig, Christoph.,Frey, Matthias.,...&Chen, Jia.(2019).Analysis of total column CO2 and CH4 measurements in Berlin with WRF-GHG.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(17),11279-11302.
MLA Zhao, Xinxu,et al."Analysis of total column CO2 and CH4 measurements in Berlin with WRF-GHG".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.17(2019):11279-11302.
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