GSTDTAP  > 地球科学
DOI10.5194/acp-19-10591-2019
Preliminary results from the FARCE 2015 campaign: multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of La Reunion
Duflot, Valentin1; 39;Connor, David J.2
2019-08-21
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:16页码:10591-10618
文章类型Article
语种英语
国家France; USA; Canada; Ireland
英文摘要

The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March-April 2015 on the tropical island of La Reunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Reunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio) aerosols and composition of clouds, with a strong focus on the Maido mountain slope area. The main observations obtained during this 2-month intensive field campaign are summarized. They include characterizations of forest structure, concentrations of VOCs and precursors emitted by forests, aerosol loading and optical properties in the planetary boundary layer (PBL), formation of new particles by nucleation of gas-phase precursors, icenucleating particles concentrations, and biological loading in both cloud-free and cloudy conditions. Simulations and measurements confirm that the Maido Observatory lies within the PBL from late morning to late evening and that, when in the PBL, the main primary sources impacting the Maido Observatory are of marine origin via the Indian Ocean and of biogenic origin through the dense forest cover. They also show that (i) the marine source prevails less and less while reaching the observatory; (ii) when in the PBL, depending on the localization of a horizontal wind shear, the Maido Observatory can be affected by air masses coming directly from the ocean and passing over the Maido mountain slope, or coming from inland; (iii) bio-aerosols can be observed in both cloud-free and cloudy conditions at the Maido Observatory; (iv) BVOC emissions by the forest covering the Maido mountain slope can be transported upslope within clouds and are a potential cause of secondary organic aerosol formation in the aqueous phase at the Maido Observatory; and (v) the simulation of dynamics parameters, emitted BVOCs and cloud life cycle in the Meso-NH model are realistic, and more advanced Meso-NH simulations should use an increased horizontal resolution (100 m) to better take into account the orography and improve the simulation of the wind shear front zone within which lies the Maido Observatory. Using various observations and simulations, this work draws up an inventory of the in situ studies that could be performed in La Reunion and at the Maido Observatory. It also aims to develop scientific collaborations and to support future scientific projects in order to better understand the forest-gas-aerosol-cloud system in an insular tropical environment.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000482493100001
WOS关键词SECONDARY ORGANIC AEROSOL ; ICE-NUCLEATING PARTICLES ; BIOGENIC EMISSIONS ; BIOLOGICAL AEROSOL ; FORMATION EVENTS ; BOUNDARY-LAYER ; INDIAN-OCEAN ; IMPACT ; CHEMISTRY ; MODEL
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/186102
专题地球科学
作者单位1.Univ la Reunion, CNRS, Lab Atmosphere & Cyclones LACy, UMR8105,Meteo France, St Denis De La Reunion, France;
2.OSUR, UMS3365, St Denis De La Reunion, France;
3.UMR PVBMT, Peuplements Vegetaux & Bioagresseurs Milieu Trop, St Denis De La Reunion, France;
4.Univ Clermont Auvergne, CNRS, Lab Meteorol Phys LaMP, F-63000 Clermont Ferrand, France;
5.NOAA, Boulder, CO USA;
6.Cooperat Inst Res Environm Sci, Boulder, CO USA;
7.Univ Denver, Dept Chem & Biochem, Denver, CO USA;
8.UC Boulder, Dept Civil & Environm Engn, Boulder, CO USA;
9.CNRS Meteo France, UMR3589, CNRM, Toulouse, France;
10.Univ British Columbia, Dept Chem, Vancouver, BC, Canada;
11.Univ Versailles St Quentin En Yvelines, CNRS, Commissariat Energie Atom & Energies Alternat, LSCE, F-91191 Gif Sur Yvette, France;
12.Univ Clermont Auvergne, CNRS, Sigma Clermont, Inst Chim Clermont Ferrand, F-63000 Clermont Ferrand, France;
13.Univ Antilles, Lab Rech Geosci & Energies LaRGE, Pointe A Pitre, Guadeloupe, France;
14.Technol Univ Dublin, Sch Chem & Pharmaceut Sci, Dublin, Ireland;
15.ATMO Occitanie, Perols, France
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GB/T 7714
Duflot, Valentin,39;Connor, David J.. Preliminary results from the FARCE 2015 campaign: multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of La Reunion[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(16):10591-10618.
APA Duflot, Valentin,&39;Connor, David J..(2019).Preliminary results from the FARCE 2015 campaign: multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of La Reunion.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(16),10591-10618.
MLA Duflot, Valentin,et al."Preliminary results from the FARCE 2015 campaign: multidisciplinary study of the forest-gas-aerosol-cloud system on the tropical island of La Reunion".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.16(2019):10591-10618.
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