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DOI10.5194/acp-19-7955-2019
Exploring aerosol-cloud interaction using VOCALS-REx aircraft measurements
Jia, Hailing1,2; Ma, Xiaoyan1,2; Liu, Yangang3
2019-06-18
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:12页码:7955-7971
文章类型Article
语种英语
国家Peoples R China; USA
英文摘要

In situ aircraft measurements obtained during the VAMOS (Variability of the American Monsoons) Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) field campaign are analyzed to study the aerosol-cloud interactions in the stratocumulus clouds over the southeastern Pacific Ocean (SEP), with a focus on three understudied topics (separation of aerosol effects from dynamic effects, dispersion effects, and turbulent entrainment-mixing processes). Our analysis suggests that an increase in aerosol concentration tends to simultaneously increase both cloud droplet number concentration (N-d) and relative dispersion (epsilon), while an increase in vertical velocity (omega) often increases N-d but decreases epsilon. After constraining the differences of cloud dynamics, the positive correlation between epsilon and N-d becomes stronger, implying that perturbations of w could weaken the aerosol influence on epsilon and hence result in an underestimation of dispersion effect. A comparative analysis of the difference of cloud microphysical properties between the entrainment and non-entrainment zones suggests that the entrainment-mixing mechanism is predominantly extremely inhomogeneous in the stratocumulus that capped by a sharp inversion, whereby the variation in liquid water content (25 %) is similar to that of N-d (29 %) and the droplet size remains approximately constant. In entrainment zone, drier air entrained from the top induces fewer cloud droplets with respect to total in-cloud particles (0.56 +/- 0.22) than the case in the non-entrainment zone (0.73 +/- 0.13) by promoting cloud droplet evaporation. This study is helpful in reducing uncertainties in dispersion effects and entrainment mixing for stratocumulus, and the results of this study may benefit cloud parameterizations in global climate models to more accurately assess aerosol indirect effects.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000472078400001
WOS关键词DROPLET SIZE DISTRIBUTION ; STRATOCUMULUS CLOUDS ; MARINE STRATOCUMULUS ; CONVECTIVE CLOUDS ; EFFECTIVE RADIUS ; BOUNDARY-LAYER ; CUMULUS CLOUD ; WARM CLOUDS ; CHEMICAL-COMPOSITION ; RADIATIVE PROPERTIES
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/184133
专题地球科学
作者单位1.Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Forecast & Evaluat Meteoro, Nanjing 210044, Jiangsu, Peoples R China;
2.Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, China Meteorol Adm, Key Lab Aerosol Cloud Precipitat, Nanjing 210044, Jiangsu, Peoples R China;
3.Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA
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Jia, Hailing,Ma, Xiaoyan,Liu, Yangang. Exploring aerosol-cloud interaction using VOCALS-REx aircraft measurements[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(12):7955-7971.
APA Jia, Hailing,Ma, Xiaoyan,&Liu, Yangang.(2019).Exploring aerosol-cloud interaction using VOCALS-REx aircraft measurements.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(12),7955-7971.
MLA Jia, Hailing,et al."Exploring aerosol-cloud interaction using VOCALS-REx aircraft measurements".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.12(2019):7955-7971.
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