Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-19-6701-2019 |
The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations | |
Lachatre, Mathieu1; Fortems-Cheiney, Audrey1,4; Foret, Gilles1; Siour, Guillaume1; Dufour, Gaelle1; Clarisse, Lieven3; Clerbaux, Cathy2,3; Coheur, Pierre-Francois3; Van Damme, Martin3; Beekmann, Matthias1 | |
2019-05-20 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2019 |
卷号 | 19期号:10页码:6701-6716 |
文章类型 | Article |
语种 | 英语 |
国家 | France; Belgium |
英文摘要 | Air pollution reaching hazardous levels in many Chinese cities has been a major concern in China over the past decades. New policies have been applied to regulate anthropogenic pollutant emissions, leading to changes in atmospheric composition and in particulate matter (PM) production. Increasing levels of atmospheric ammonia columns have been observed by satellite during recent years. In particular, observations from the Infrared Atmospheric Sounding Interferometer (IASI) reveal an increase of these columns by 15 % and 65 % from 2011 to 2013 and 2015, respectively, over eastern China. In this paper we performed model simulations for 2011, 2013 and 2015 in order to understand the origin of this increase and to quantify the link between ammonia and the inorganic components of particles: NH4(P)+/SO4(p)2-/NO3(p)-. Interannual change of meteorology 3 can be excluded as a reason: year 2015 meteorology leads to enhanced sulfate production over eastern China, which increases the ammonium and decreases the ammonia content, which is contrary to satellite observations. Reductions in SO2 and NOx emissions from 2011 to 2015 of 37.5 % and 21 % respectively, as constrained from satellite data, lead to decreased inorganic matter (by 14 % for NH4(P)+/SO4(p)2-/NO3(p)-). This in turn leads to increased 4(p) P gaseous NH3(g) tropospheric columns by as much as 24 % and 49 % (sampled corresponding to IASI data availability) from 2011 to 2013 and 2015 respectively and thus can explain most of the observed increase. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000468419100001 |
WOS关键词 | NITROGEN-OXIDES ; AIR-POLLUTION ; EMISSION CHANGES ; SULFUR-DIOXIDE ; TRENDS ; AEROSOLS ; MODEL ; VARIABILITY ; INVENTORIES ; TRANSPORT |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/183313 |
专题 | 地球科学 |
作者单位 | 1.Univ Paris, Univ Paris Est Creteil, Inst Pierre Simon Laplace, UMR7583,CNRS,LISA, Creteil, France; 2.Sorbonne Univ, UVSQ, CNRS, LATMOS,IPSL, Paris, France; 3.Univ Libre Bruxelles, Spect Atmospher, Serv Chim Quant & Photophys, Brussels, Belgium; 4.Univ Paris Saclay, UVSQ, LSCE, IPSL,CEA,CNRS, F-91191 Gif Sur Yvette, France |
推荐引用方式 GB/T 7714 | Lachatre, Mathieu,Fortems-Cheiney, Audrey,Foret, Gilles,et al. The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(10):6701-6716. |
APA | Lachatre, Mathieu.,Fortems-Cheiney, Audrey.,Foret, Gilles.,Siour, Guillaume.,Dufour, Gaelle.,...&Beekmann, Matthias.(2019).The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(10),6701-6716. |
MLA | Lachatre, Mathieu,et al."The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.10(2019):6701-6716. |
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