Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1029/2018JD029892 |
Optical Properties of Laboratory and Ambient Biomass Burning Aerosols: Elucidating Black, Brown, and Organic Carbon Components and Mixing Regimes | |
Romonosky, Dian E.1; Gomez, Samantha L.1,2; Lam, Jared2; Carrico, Christian M.2; Aiken, Allison C.1; Chylek, Petr1; Dubey, Manvendra K.1 | |
2019-05-16 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES |
ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2019 |
卷号 | 124期号:9页码:5088-5105 |
文章类型 | Article |
语种 | 英语 |
国家 | USA |
英文摘要 | Biomass burning (BB) is an important global source of aerosol and trace gases that degrade air quality, decrease visibility, and impact climate and human health. Refractory black carbon (rBC), brown carbon (BrC), and organic aerosol are major components of BB emissions. BB aerosol composition is highly variable at the source and depends on fuel composition and combustion phase. Atmospheric aging alters fresh BB aerosol through processes that are complex and dynamic. To better understand the variability in optical properties, we report fresh aerosol laboratory measurements from burning southwestern U.S. fuels and compare them to aged ambient BB aerosol from wildfires over a range of atmospheric time scales. Our BB aerosol analysis uses the relationship between the absorption angstrom ngstrom exponent and single-scattering albedo (SSA) to identify rBC, BrC, and organic aerosol-dominated regimes that are defined using Mie theory. This model framework is used to interpret the large variability in optical properties measured in laboratory burns. In contrast, we find the observed absorption angstrom ngstrom exponent-SSA relationship for ambient BB aerosol to be less variable and more clustered together with increased atmospheric aging. This transition from fresh to aged behavior is attributed to the homogenization of the BB aerosol from mixing and aging over several hours. Finally, BB aerosol in ambient fire plumes that have aged for several hours exhibits larger SSAs than laboratory flaming burns. We conclude that BrC/OC mixtures play a larger role than rBC in the positive climate forcing of BB aerosol than what would be projected from laboratory results. |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000469175600014 |
WOS关键词 | ABSORPTION ANGSTROM EXPONENT ; ATMOSPHERIC TAR BALLS ; LIGHT-ABSORPTION ; PHOTOACOUSTIC SPECTROMETER ; WAVELENGTH DEPENDENCE ; SPECTRAL DEPENDENCE ; PHYSICAL-PROPERTIES ; CAVITY RING ; SOOT ; SCATTERING |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/183298 |
专题 | 气候变化 |
作者单位 | 1.Los Alamos Natl Lab, Earth & Environm Sci Div, Los Angeles, CA 87545 USA; 2.New Mexico Inst Min & Technol, Dept Civil & Environm Engn, Socorro, NM 87801 USA |
推荐引用方式 GB/T 7714 | Romonosky, Dian E.,Gomez, Samantha L.,Lam, Jared,et al. Optical Properties of Laboratory and Ambient Biomass Burning Aerosols: Elucidating Black, Brown, and Organic Carbon Components and Mixing Regimes[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2019,124(9):5088-5105. |
APA | Romonosky, Dian E..,Gomez, Samantha L..,Lam, Jared.,Carrico, Christian M..,Aiken, Allison C..,...&Dubey, Manvendra K..(2019).Optical Properties of Laboratory and Ambient Biomass Burning Aerosols: Elucidating Black, Brown, and Organic Carbon Components and Mixing Regimes.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,124(9),5088-5105. |
MLA | Romonosky, Dian E.,et al."Optical Properties of Laboratory and Ambient Biomass Burning Aerosols: Elucidating Black, Brown, and Organic Carbon Components and Mixing Regimes".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 124.9(2019):5088-5105. |
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