GSTDTAP  > 气候变化
DOI10.1029/2019GL082172
The 2005-2016 Trends of Formaldehyde Columns Over China Observed by Satellites: Increasing Anthropogenic Emissions of Volatile Organic Compounds and Decreasing Agricultural Fire Emissions
Shen, Lu1; Jacob, Daniel J.1; Zhu, Lei1,2; Zhang, Qiang3; Zheng, Bo4; Sulprizio, Melissa P.1; Li, Ke1; De Smedt, Isabelle5; Abad, Gonzalo Gonzalez2; Cao, Hansen6; Fu, Tzung-May7; Liao, Hong8
2019-04-28
发表期刊GEOPHYSICAL RESEARCH LETTERS
ISSN0094-8276
EISSN1944-8007
出版年2019
卷号46期号:8页码:4468-4475
文章类型Article
语种英语
国家USA; Peoples R China; France; Belgium
英文摘要

We use 2005-2016 observations of formaldehyde (HCHO) columns over China from the OMI, GOME-2, and SCIAMACHY satellite instruments to evaluate long-term trends in emission inventories of volatile organic compounds (V005) that affect air quality. The observations show large increases over 2005-2016 in the North China Plain (+1.1 +/- 0.5% a(-1) relative to 2005) and the Yangtze River Delta region (+1.5 +/- 0.4% a(-1) relative to 2005), consistent with the trend of anthropogenic VOC emissions in the Multi-resolution Emission Inventory for China (MEIC). Unlike other pollutants, VOC emissions have not been decreasing in recent years. An exception is the Huai River Basin in rural eastern China where the satellite data show rapidly decreasing VOC emissions since the early 2010s that appear to reflect bans on agricultural fires.


Plain Language Summary Satellite observations of formaldehyde can detect emissions of volatile organic compounds (V005), which are of concern for air quality. Here we use 2005-2016 satellite observations of formaldehyde over China to infer trends in VOC emissions. We find increases of 13% in the North China Plain and 18% in the Yangtze River Delta. Unlike other pollutants, emissions of VOCs in China have not decreased in recent years. An exception is in rural areas where post-2010 restrictions on crop burning to improve air quality have resulted in sharp decreases of VOC emissions.


领域气候变化
收录类别SCI-E
WOS记录号WOS:000467949200044
WOS关键词MAX-DOAS OBSERVATIONS ; ISOPRENE EMISSIONS ; TROPOSPHERIC OZONE ; NORTH-AMERICA ; OMI ; HCHO ; AEROSOLS ; MODEL ; SPACE ; VALIDATION
WOS类目Geosciences, Multidisciplinary
WOS研究方向Geology
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/182531
专题气候变化
作者单位1.Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA;
2.Harvard Smithsonian Ctr Astrophys, Atom & Mol Phys Div, 60 Garden St, Cambridge, MA 02138 USA;
3.Tsinghua Univ, Minist Educ, Key Lab Earth Syst Modeling, Dept Earth Syst Sci, Beijing, Peoples R China;
4.CEA CNRS UVSQ, Lab Sci Climat & Environm, UMR8212, Gif Sur Yvette, France;
5.Belgian Inst Space Aeron BIRA IASB, Brussels, Belgium;
6.Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA;
7.Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Beijing, Peoples R China;
8.Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Nanjing, Jiangsu, Peoples R China
推荐引用方式
GB/T 7714
Shen, Lu,Jacob, Daniel J.,Zhu, Lei,et al. The 2005-2016 Trends of Formaldehyde Columns Over China Observed by Satellites: Increasing Anthropogenic Emissions of Volatile Organic Compounds and Decreasing Agricultural Fire Emissions[J]. GEOPHYSICAL RESEARCH LETTERS,2019,46(8):4468-4475.
APA Shen, Lu.,Jacob, Daniel J..,Zhu, Lei.,Zhang, Qiang.,Zheng, Bo.,...&Liao, Hong.(2019).The 2005-2016 Trends of Formaldehyde Columns Over China Observed by Satellites: Increasing Anthropogenic Emissions of Volatile Organic Compounds and Decreasing Agricultural Fire Emissions.GEOPHYSICAL RESEARCH LETTERS,46(8),4468-4475.
MLA Shen, Lu,et al."The 2005-2016 Trends of Formaldehyde Columns Over China Observed by Satellites: Increasing Anthropogenic Emissions of Volatile Organic Compounds and Decreasing Agricultural Fire Emissions".GEOPHYSICAL RESEARCH LETTERS 46.8(2019):4468-4475.
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