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DOI | 10.5194/acp-18-16747-2018 |
Aerosol water parameterization: long-term evaluation and importance for climate studies | |
Metzger, Swen1,2,3; Abdelkader, Mohamed1,2,4; Steil, Benedikt2; Klingmueller, Klaus2 | |
2018-11-27 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:22页码:16747-16774 |
文章类型 | Article |
语种 | 英语 |
国家 | Cyprus; Germany; Saudi Arabia |
英文摘要 | We scrutinize the importance of aerosol water for the aerosol optical depth (AOD) calculations using a long-term evaluation of the EQuilibrium Simplified Aerosol Model v4 for climate modeling. EQSAM4clim is based on a single solute coefficient approach that efficiently parameterizes hygroscopic growth, accounting for aerosol water uptake from the deliquescence relative humidity up to supersaturation. EQSAM4clim extends the single solute coefficient approach to treat water uptake of multicomponent mixtures. The gas-aerosol partitioning and the mixed-solution water uptake can be solved analytically, preventing the need for iterations, which is computationally efficient. EQSAM4clim has been implemented in the global chemistry climate model EMAC and compared to ISORROPIA II on climate timescales. Our global modeling results show that (I) our EMAC results of the AOD are comparable to modeling results that have been independently evaluated for the period 2000-2010, (II) the results of various aerosol properties of EQSAM4clim and ISORROPIA II are similar and in agreement with AERONET and EMEP observations for the period 2000-2013, and (III) the underlying assumptions on the aerosol water uptake limitations are important for derived AOD calculations. Sensitivity studies of different levels of chemical aging and associated water uptake show larger effects on AOD calculations for the year 2005 compared to the differences associated with the application of the two gas-liquid-solid partitioning schemes. Overall, our study demonstrates the importance of aerosol water for climate studies. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000451273900003 |
WOS关键词 | THERMODYNAMIC-EQUILIBRIUM MODEL ; TECHNICAL NOTE ; PARTICULATE MATTER ; CONVECTION PARAMETERISATIONS ; HYGROSCOPIC GROWTH ; DUST EMISSIONS ; MINERAL DUST ; CHEMISTRY ; SUBMODEL ; SENSITIVITY |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/17244 |
专题 | 地球科学 |
作者单位 | 1.Cyprus Inst, Energy Environm & Water Res Ctr, Nicosia, Cyprus; 2.Max Planck Inst Chem, Air Chem Dept, Mainz, Germany; 3.ResearchConcepts Io GmbH, Freiburg, Germany; 4.King Abdullah Univ Sci & Technol, Thuwal, Saudi Arabia |
推荐引用方式 GB/T 7714 | Metzger, Swen,Abdelkader, Mohamed,Steil, Benedikt,et al. Aerosol water parameterization: long-term evaluation and importance for climate studies[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(22):16747-16774. |
APA | Metzger, Swen,Abdelkader, Mohamed,Steil, Benedikt,&Klingmueller, Klaus.(2018).Aerosol water parameterization: long-term evaluation and importance for climate studies.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(22),16747-16774. |
MLA | Metzger, Swen,et al."Aerosol water parameterization: long-term evaluation and importance for climate studies".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.22(2018):16747-16774. |
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