Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1016/j.atmosres.2016.08.014 |
Metal-bearing fine particle sources in a coastal industrialized environment | |
Mbengue, Saliou1,2,4; Alleman, Laurent Y.1,2; Flament, Pascal3 | |
2017 | |
发表期刊 | ATMOSPHERIC RESEARCH |
ISSN | 0169-8095 |
EISSN | 1873-2895 |
出版年 | 2017 |
卷号 | 183 |
文章类型 | Article |
语种 | 英语 |
国家 | France; Czech Republic |
英文摘要 | Fine (<2.5 mu m), submicron (<1 mu m) and ultrafine (<100 nm) atmospheric particles were collected during a 3 weeks campaign in a heavily industrialized area and physically and chemically characterized in order to determine their main sources. As a basis of comparison, the present one-year average EU limit value (25 mu g.m(-3)) and the WHO recommendation for PM2.5 (10 mu g m(-3)) were regularly exceeded during this campaign. Submicron particles (PM1) account for 55 to 70% of PM2.5 mass concentrations. A bi-modal size distribution, centered on 0.4 and 2.0 mu m, suggests two types of emissions: high temperature processes that liberate primary or secondary sub micron particles and mechanical procedures in open air, or local traffic, which lead to the emission of coarser particles (>1 mu m). The trace elements As, Cd, Ni, Pb, Sb, V and Zn, characteristics of the local industrial activities display 60% to 85% of their mass in the submicron and ultrafine fractions and appear highly enriched, by reference to the crustal source. High atmospheric pressure periods, corresponding to northeasterly winds, induce the highest contributions of metalworking emissions and the highest PM2.5 concentrations (32.5 +/- 11.9 mu g. m(-3)). A Principal Component Analysis of the dataset produces 7 factors associated to metallurgy-, steelworks-, oil processing-, coal combustion-, neighboring traffic-, dust resuspension- and sea salt-sources, that explain the obtained concentrations. A Multiple Linear Regression Analysis confirms that Fe-Mn alloy refining, iron-and steel-making are the main sources (>40%) controlling metal concentrations in PM2.5. Less predictably, resuspended dust and fresh/aged sea salts are also significant contributors (approximate to 20%). Considering the related health hazards, authorities should pay more attention to the exposure of people living in this area and the possible impact of fine particles in terms of public health. (C) 2016 Elsevier B.V. All rights reserved. |
英文关键词 | PM2.5 Trace elements Industrial emissions Sources apportionment |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000386861800017 |
WOS关键词 | ULTRAFINE ATMOSPHERIC PARTICLES ; PARTICULATE MATTER ; SOURCE APPORTIONMENT ; CHEMICAL-CHARACTERIZATION ; TRACE-ELEMENTS ; AIR-POLLUTION ; AMBIENT AIR ; EMISSIONS ; URBAN ; VICINITY |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/15292 |
专题 | 地球科学 |
作者单位 | 1.Mines Douai, SAGE, CS10838, F-59508 Douai, France; 2.Univ Lille, Lille, France; 3.ULCO, LPCA, 189A Ave Maurice Schumann, F-59240 Dunkerque, France; 4.Czech Acad Sci, Global Change Res Inst, Brno, Czech Republic |
推荐引用方式 GB/T 7714 | Mbengue, Saliou,Alleman, Laurent Y.,Flament, Pascal. Metal-bearing fine particle sources in a coastal industrialized environment[J]. ATMOSPHERIC RESEARCH,2017,183. |
APA | Mbengue, Saliou,Alleman, Laurent Y.,&Flament, Pascal.(2017).Metal-bearing fine particle sources in a coastal industrialized environment.ATMOSPHERIC RESEARCH,183. |
MLA | Mbengue, Saliou,et al."Metal-bearing fine particle sources in a coastal industrialized environment".ATMOSPHERIC RESEARCH 183(2017). |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论